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- W4382140699 abstract "The stoichiometric water splitting using a solar-driven Z-scheme approach is an emerging field of interest to address the increasing renewable energy demand and environmental concerns. So far, the reported Z-scheme must comprise two populations of photocatalysts. In the present work, only tungsten oxides are used to construct a robust Z-scheme system for complete visible-driven water splitting in both neutral and alkaline solutions, where sodium tungsten oxide bronze (Na0.56WO3-x) is used as a H2 evolution photocatalyst and two-dimensional (2D) tungsten trioxide (WO3) nanosheets as an O2 evolution photocatalyst. This system efficiently produces H2 (14 μmol h-1) and O2 (6.9 μmol h-1) at an ideal molar ratio of 2:1 in an aqueous solution driven by light, resulting in a remarkably high apparent quantum yield of 6.06% at 420 nm under neutral conditions. This exceptional selective H2 and O2 production is due to the preferential adsorption of iodide (I-) on Na0.56WO3-x and iodate (IO3-) on WO3, which is evidenced by both experiments and density functional theory calculation. The present liquid Z-scheme in the presence of efficient shuttle molecules promises a separated H2 and O2 evolution by applying a dual-bed particle suspension system, thus a safe photochemical process." @default.
- W4382140699 created "2023-06-27" @default.
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- W4382140699 date "2023-06-26" @default.
- W4382140699 modified "2023-10-14" @default.
- W4382140699 title "Tungsten Oxide-Based Z-Scheme for Visible Light-Driven Hydrogen Production from Water Splitting" @default.
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- W4382140699 doi "https://doi.org/10.1021/acscatal.3c01312" @default.
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