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• W4382248663 abstract "Ultrasmall silver clusters in reduced state are difficult to synthesize since silver atoms tend to rapidly aggregate into bigger entities. Here, we show that dimers of reduced silver (Ag2) are formed within the framework of a metal-organic framework provided with thioether arms in their walls (methioMOF), after reduction with NaBH4 of the corresponding Ag+-methioMOF precursor. The resulting Ag2-methioMOF catalyzes the methanation reaction of carbon dioxide (CO2 to CH4 hydrogenation reaction) under mild reaction conditions (1 atm CO2, 4 atm H2, 140 °C), with production rates much higher than Ag on alumina and even comparable to the state-of-the-art Ru on alumina catalyst (Ru-Al2O3) under these reaction conditions, according to literature results." @default.
• W4382248663 created "2023-06-28" @default.
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• W4382248663 date "2023-06-27" @default.
• W4382248663 modified "2023-10-18" @default.
• W4382248663 title "Ag2(0) dimers within a thioether-functionalized MOF catalyze the CO2 to CH4 hydrogenation reaction" @default.
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• W4382248663 doi "https://doi.org/10.1038/s41598-023-37600-4" @default.
• W4382248663 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37369737" @default.
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