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• W4382364216 abstract "Copper organic complexes with strong chemical stability and high solubility in water are difficult to eliminate with traditional adsorbents. In this work, a novel amidoxime nanofiber (AO-Nanofiber) with the p-π conjugated structure was fabricated through homogeneous chemical grafting coupled with electrospinning and applied to capture cupric tartrate (Cu-TA) from aqueous solutions. The adsorption capacity of Cu-TA by AO-Nanofiber was 198.4 mg/g at an equilibrium time of 40 min, and the adsorption performance remains basically unchanged after 10 times adsorption-desorption cycles. The capture mechanism of Cu-TA by AO-Nanofiber was jointly validated by experiments and characterization such as Fourier Transform Infrared Spectrometer (FT-IR), X-ray Photoelectron Spectroscopy (XPS), and Density functional theory (DFT) calculations. These results demonstrated that the lone pair of electrons of the N atom from the amino groups and the O atom from hydroxyl groups in the AO-Nanofiber is partially transferred to the 3d orbital of the Cu(II) ions in Cu-TA, leading to the Jahn-Teller distortion of the Cu-TA and the more stable structure of AO-Nanofiber@Cu-TA was generated." @default.
• W4382364216 created "2023-06-29" @default.
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• W4382364216 date "2023-11-01" @default.
• W4382364216 modified "2023-10-12" @default.
• W4382364216 title "A nanofiber with a p-π conjugated structure designed based on the Jahn-Teller effect for the removal of cupric tartrate from wastewater" @default.
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• W4382364216 doi "https://doi.org/10.1016/j.jcis.2023.06.195" @default.
• W4382364216 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37399752" @default.
• W4382364216 hasPublicationYear "2023" @default.
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