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- W4382517355 abstract "<strong class=journal-contentHeaderColor>Abstract.</strong> In this manuscript, we provide an analytical description of the performance of the cross-polarization experiment, including linear ramp and adiabatic tangential sweep modifications, using effective Hamiltonians and simple rotations in 3D space. It is shown that radiofrequency field inhomogeneity induces a reduction of the transfer efficiency at increasing MAS frequencies for both the ramp and the adiabatic CP experiments. The effect depends on the ratio of the dipolar coupling constant and the sample rotation frequency. In particular, our simulations show that for small dipolar couplings (1 kHz) and ultrafast MAS (above 100 kHz) the transfer efficiency is below 40 % when extended contact times up to 20 ms are used and relaxation losses are ignored. New recoupling and magnetization transfer techniques that are designed explicitly to account for inhomogeneous RF fields are needed." @default.
- W4382517355 created "2023-06-30" @default.
- W4382517355 creator A5082967525 @default.
- W4382517355 date "2023-06-29" @default.
- W4382517355 modified "2023-10-02" @default.
- W4382517355 title "Reply on RC3" @default.
- W4382517355 doi "https://doi.org/10.5194/mr-2023-9-ac4" @default.
- W4382517355 hasPublicationYear "2023" @default.
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