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- W4382561138 abstract "Kink sites play a pivotal role in the growth and dissolution of materials at the solid-liquid interface. Despite this, little is known about the thermodynamic stability of such sites. Calcium carbonate, in the form of calcite, is one of the most abundant biominerals and a natural means of carbon sequestration in the environment. Here we present a complete determination of the standard free energies for all 16 individual kink sites for the significant case of the calcite (10-14)--water interface using both alchemical and pathway-based simulation techniques. The results reveal the importance of distinguishing between real and ideal ion-binding free energies at surfaces, especially for calcite-water where the interfacial potential can alter values by more than 100 kJ/mol per site. Individual kink site stabilities are found to show variations in excess of 60 kJ/mol, which can help explain observed differences in growth rates between the two distinct steps of calcite." @default.
- W4382561138 created "2023-06-30" @default.
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- W4382561138 date "2023-06-29" @default.
- W4382561138 modified "2023-09-27" @default.
- W4382561138 title "Determining the Complete Stability of Calcite Kink Sites: Real vs Ideal" @default.
- W4382561138 doi "https://doi.org/10.26434/chemrxiv-2023-g9kc9-v2" @default.
- W4382561138 hasPublicationYear "2023" @default.
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