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- W4382877617 abstract "A series of modified biochar with hierarchical pore structures (ZnxBC1, x = 0.5, 1, 2, 3) was obtained by ZnCl2 and investigated the adsorption performance of sulfamethoxazole (SMX). The structure and composition of ZnxBC1 were well characterized by the material analysis technique. Compared with unmodified biochar (BC), the specific surface area, pore volume, and adsorption capacity of ZnxBC1 significantly increased. The ZnxBC1 performed a significant adsorption capacity of SMX with the maximum adsorption amount of 597.57 mg/g, leading to a 54-fold increase in that of BC (11.04 mg/g). Multiple linear regression analysis showed that the quantitative relationship of qe with Vmeso and Vmicro was qe = 360.74*Vmeso + 871.58*Vmicro-22.26, which was the novelty of the study to the analysis of SMX adsorption capacity on the different Vmeso/Vmicro ratios of adsorbents. Based on the batch experiment results, an artificial neural network (ANN) model with a topology of 5:5:10:1 was developed to sufficiently describe the adsorption data (R2 > 0.99), and possessed good predictability in different water quality conditions. Additionally, both static adsorption and dynamic adsorption experiments of Zn1BC1 showed excellent regeneration properties. Overall, the ZnCl2 modified biochar with the properties of rapid adsorption rate, high adsorption capacity, multiple reuses, and low-cost performed the potential utilization for the removal of SMX, and the effect of pore structure of biochar on SMX adsorption could guide the design and preparation of efficient antibiotics adsorbents." @default.
- W4382877617 created "2023-07-02" @default.
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- W4382877617 date "2023-08-01" @default.
- W4382877617 modified "2023-09-30" @default.
- W4382877617 title "Characteristics and mechanisms of sulfamethoxazole adsorption onto modified biochars with hierarchical pore structures: Batch, predictions using artificial neural network and fixed bed column studies" @default.
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- W4382877617 doi "https://doi.org/10.1016/j.jwpe.2023.103975" @default.
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