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- W4382891128 abstract "A novel thermodynamic theory of the properties of supercooled liquids as they get glassy is presented. It is based on the postulated existence of a narrowly avoided thermodynamic phase transition at a temperature T∗ ⩾ Tm, where Tm is the melting point, and the “avoidance” is due to geometric frustration. We show that as a consequence two large emergent length scales develop at temperatures less than T∗, and we also show that this picture is consistent with appropriate statistical mechanical models. A theoretical expression is obtained which permits collapse of the viscosity versus temperature of all known glass-formers onto a single master-curve." @default.
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- W4382891128 date "1995-09-01" @default.
- W4382891128 modified "2023-10-16" @default.
- W4382891128 title "A thermodynamic theory of supercooled liquids" @default.
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- W4382891128 doi "https://doi.org/10.1016/0378-4371(95)00140-3" @default.
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