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- W4383163261 abstract "Understanding the impact of abundant inherent moisture in sewage sludge on the physicochemical properties and adsorption applications of sludge-derived biochar (SDB) contributed significantly to promoting economical sludge reuse. The moisture (0–80%) contributed to the development of micropore and mesopore in SDB at 400 °C, resulting in a maximum increase in specific surface area (SSA) and total pore volume (TPV) of SDB by 38.47% (84.811–117.437 m2/g) and 92.60% (0.0905–0.1743 m3/g), respectively. At 600/800 °C, moisture only facilitated mesopore formation, while was exacerbated with increasing moisture content. Despite reduction in SSA during this stage, TPV increased by a maximum of 20.47% (0.1700–0.2048 m3/g). The presence of moisture during pyrolysis led to an increase in the formation of 3–5 thickened benzene rings and defective structures in SDB, along with more C=O, O–C=O/–OH, pyrrole N, pyridine N, and thiophene. As a result, moisture (40%/80%) increased the maximum adsorption capacity (76.2694–88.0448/90.1190 mg/g) of SDB (600 °C) for tetracycline, mainly due to enhanced pore filling effect and hydrogen bonding induced by improved physicochemical properties. This study offered a novel approach for optimizing the performance of SDB adsorption applications by manipulating the sludge moisture, which is critical for practical sludge management." @default.
- W4383163261 created "2023-07-05" @default.
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- W4383163261 date "2023-09-01" @default.
- W4383163261 modified "2023-10-18" @default.
- W4383163261 title "Optimizing adsorption performance of sludge-derived biochar via inherent moisture-regulated physicochemical properties" @default.
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- W4383163261 doi "https://doi.org/10.1016/j.wasman.2023.06.033" @default.
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