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- W4383265925 abstract "Abstract Metallopolymers (MEPEs) show a strong absorption band attributed to a metal‐to‐ligand charge transfer (MLCT) transition. Fe‐MEPE and Ru‐MEPE thin films switch reversibly from blue‐purple (λ max =584 nm, Fe 2+ ) to colorless (Fe 3+ ) or orange (λ max =518 nm, Ru 2+ ) to pale green (Ru 3+ ). The addition of multi‐walled carbon nanotubes (MWCNTs) enhances the electrochromic (EC) properties of Fe‐ and Ru‐MEPE electrodes in several ways: (1) faster response for bleaching/coloring; (2) enhanced Coulombic efficiency; and (3) improved cycling stability, particularly for Ru‐MEPE. Moreover, the charge density of the thin film electrodes can be increased upon the addition of the MWCNTs. This performance improvement is demonstrated in electrochromic devices (ECDs) with titanium‐doped vanadium oxide (TiVO x ) as the optically‐passive ion storage layer. The visible light transmittance τ v values of the ECDs are improved by the addition of the MWCNTs from 20 %/56 % to 17 %/56 % and from 31 %/47 % and 34 %/55 % in the dark/bright state, for Fe‐MEPE and Ru‐MEPE, respectively. Thus, the addition of MWCNTs to Fe‐ or Ru‐MEPE is a very promising route for future fast‐switching EC applications, e. g., displays, sunroofs, and rear‐view mirrors." @default.
- W4383265925 created "2023-07-06" @default.
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- W4383265925 date "2023-07-05" @default.
- W4383265925 modified "2023-10-14" @default.
- W4383265925 title "Addition of Multi‐walled Carbon Nanotubes to Fe‐ and Ru‐Metallopolymer Electrodes Enhances Response Time and Cycling Stability in Electrochromic Cells" @default.
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- W4383265925 doi "https://doi.org/10.1002/celc.202300178" @default.
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