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- W4383620793 abstract "Abstract Organic cathodes for aqueous zinc‐ion batteries (AZIBs) feature intrinsic flexibility and favorable kinetics, but they suffer from high solubility. Herein, a partial charge regulation strategy is deployed by designing a small organic molecule with extended π ‐conjugated plane, namely benzo[i]benzo[6′,7′]quinoxalino[2′,3′:9,10]phenanthro[4,5‐abc]phenazine‐5,10,16,21‐tetraone (PTONQ). The charge equalization of active sites induced by the extended π ‐conjugated plane of the PTONQ molecule combined with high aromaticity renders the molecule low solubility, fast charge transfer, and high structural stability. The fabricated Zn//PTONQ battery cycles more than 500 h at 175 mA g −1 with small capacity reduction, fast charged/discharged kinetics, and anti‐freeze performance (below ‐20°C). By a series of ex situ characterizations, it is attested that the capacity originates mainly from Zn 2+ insertion/removal of PTONQ without H + incorporation, which also accounts for the formation of Zn x (CF 3 SO 3 ) y (OH) 2x‐y ·nH 2 O by‐products. This result benefits the understanding of the by‐product formation mechanism of organic cathode and paves a new way to advance the aqueous Zn‐organic batteries." @default.
- W4383620793 created "2023-07-09" @default.
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- W4383620793 date "2023-07-08" @default.
- W4383620793 modified "2023-10-17" @default.
- W4383620793 title "Dynamic Balance of Partial Charge for Small Organic Compound in Aqueous Zinc‐Organic Battery" @default.
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- W4383620793 doi "https://doi.org/10.1002/adfm.202306675" @default.
- W4383620793 hasPublicationYear "2023" @default.
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