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- W4383710356 abstract "The development of hierarchically porous metal–organic frameworks (MOFs) with high stability is desirable to expand their applications but remains challenging. Herein, an anionic sodalite-type microporous MOF (Yb-TTCA; TTCA3– = triphenylene-2,6,10-tricarboxylate) was synthesized, which shows outstanding catalytic activities for the cycloaddition of CO2 into cyclic carbonates. Moreover, the microporous Yb-TTCA can be transformed into a hierarchical micro- and mesoporous Yb-TTCA by water treatment with the mesopore sizes of 2 to 12 nm. The hierarchically porous Yb-TTCA (HP-Yb-TTCA) not only exhibits a high thermal stability up to 500 °C but also shows a high chemical stability in aqueous solutions with pH values ranging from 2 to 12. In addition, the HP-Yb-TTCA displays enhanced performance for the removal of organic dyes in comparison with microporous Yb-TTCA. This work provides a facile way to construct hierarchically porous MOF materials." @default.
- W4383710356 created "2023-07-11" @default.
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- W4383710356 date "2023-07-10" @default.
- W4383710356 modified "2023-10-15" @default.
- W4383710356 title "Water-Etched Approach to Hierarchically Porous Metal–Organic Frameworks with High Stability" @default.
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- W4383710356 doi "https://doi.org/10.1021/acs.inorgchem.3c01351" @default.
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