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• W4383737854 abstract "The manufacturing of thin‐films with structured surfaces by large‐scale rolling has distinct advantages over other techniques, such as lithography, due to scalability. However, it is not well understood or quantified how processing conditions can affect the microstructure at different physical scales. Hence, the objective of this investigation is to develop a validated computational model of the symmetric forward‐roll coating process to understand, predict, and control the morphology of carbon nanotubes (CNT)‐PDMS pastes. The effects of the thin‐film rheological properties and the roller gap on the ribbing behavior were investigated and a ribbing instability prediction model was formulated from experimental measurements and computational predictions. The CNT‐PDMS thin‐film system was modeled by a nonlinear implicit dynamic finite‐element (FE) method that accounted for ribbing instabilities, large displacements, rolling contact, and material viscoelasticity. Dynamic mechanical analysis was used to obtain the viscoelastic properties of the CNT‐PDMS paste for various CNT weight distributions. Furthermore, a Morris sensitivity analysis was conducted to obtain insights on the dominant predicted characteristics pertaining to the ribbing microstructure. Based on the sensitivity analysis, a critical ribbing aspect ratio was identified for the CNT‐PDMS system corresponding to a critical roller gap. This article is protected by copyright. All rights reserved." @default.
• W4383737854 created "2023-07-11" @default.
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• W4383737854 date "2023-07-09" @default.
• W4383737854 modified "2023-10-16" @default.
• W4383737854 title "Predicting and Controlling Ribbing Instabilities of Carbon Nanotube‐PDMS Thin‐Film Systems for Multifunctional Applications" @default.
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• W4383737854 doi "https://doi.org/10.1002/adem.202300582" @default.
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