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- W4383874187 abstract "Bimetallic palladium-iron (Pd-Fe) nanoparticles encapsulated in the graphitic shell of nitrogen-doped carbon nanotubes (NCNTs) (Pd56-Fe44/NCNTs) are developed via a facile chemical vapor deposition technique using the Pd-Fe nanoparticles-decorated mesoporous silica nanoparticles (MSNs) as catalytic systems. The impact of the MSN template over the formation of Pd-Fe nanoparticles and the consequent Pd-Fe/NCNT is analyzed with variant morphological and structural characterizations. Pd-Fe nanoparticles encased in NCNT tips catalytically actuate the external graphitic layers via the bimetallic synergism and accelerate the swift electron mobility, stimulating the surface reactivity of graphitic layers. With the combinatorial arrays of aligned porous carbon walls and their metal-like behavior, and bimetallic alliances, Pd56-Fe44/NCNT/CC-equipped microfluidic DEGFCs (μDEGFCs) actualize the maximal power output of 96.2 mW cm–2, while the encased Pd-Fe nanoparticles with closed carbon shells elevate the durability to 100 h. Thus, the state-of-the-art combination of porous carbon nanoarchitectures and bimetallic active sites in the Pd56-Fe44/NCNT accelerate the high DEGFC power output and durability among the reported catalysts, substantiating the prospect to cater the next-generation μDEGFCs for portable electronic devices." @default.
- W4383874187 created "2023-07-12" @default.
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- W4383874187 date "2023-07-11" @default.
- W4383874187 modified "2023-09-25" @default.
- W4383874187 title "Carbon Shell-Confined Pd-Fe Bimetallic Nanoparticles in NCNTs as Anode Catalysts for Microfluidic Direct Ethylene Glycol Fuel Cells" @default.
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- W4383874187 doi "https://doi.org/10.1021/acsaem.3c00790" @default.
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