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- W4383888051 abstract "The exploration of efficient, stable, and inexpensive oxygen evolution reaction (OER) catalysts is of great importance for the practical application of seawater electrolysis. In this work, CoSe2@CoO/CF catalysts are prepared by a simple and scalable one-step electrodeposition method, and the OER performance of the catalysts is investigated in depth. The CoSe2@CoO/CF catalyst (273 mV) shows significantly better activity than the IrO2 catalyst (435 mV). The catalyst can be steadily operated at high current densities (100 mA cm−2) for over 200 h in the 1.0 M KOH + seawater. Notably, the catalyst exhibits excellent selectivity with a Faraday efficiency of approximately 98% for OER, while the ClO− concentration is only 1.312×10−7 mol L−1 as measured by UV-visible characterization. Strong overlap between the Co 2p orbitals of monometallic bi-compound catalysts facilitates the rate of para-site electron transfer. In addition, the impressive performance is attributed to the urchin-like heterogeneous structure with abundant active centers." @default.
- W4383888051 created "2023-07-12" @default.
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- W4383888051 date "2023-09-01" @default.
- W4383888051 modified "2023-10-14" @default.
- W4383888051 title "Self-assembled heterojunction CoSe2@CoO catalysts for efficient seawater electrolysis" @default.
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- W4383888051 doi "https://doi.org/10.1016/j.electacta.2023.142870" @default.
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