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- W4383888081 abstract "Rechargeable aqueous zinc-ion hybrid supercapacitors (ZHSs) are drawing extensive attention because of their cost-effectiveness and diminished safety hazards. Nevertheless, large-scale application of ZHSs has been hindered by the severe side reactions and rampant dendrites growth on the surface of Zn metal anodes. Herein, we propose a three-dimensional organic-inorganic composite frame material as an artificial bi-functional layer coated on the zinc foil, featuring nitrogenous functional groups with zincophilicity (abbreviated as [email protected]). The nitrogen (N) site's strong adsorption capacity and synergistic effect of the sub-nanopore size promote rapid desolvation of zinc ions and reduce side reactions, while also prolonging galvanized nucleation's Sand's time and allowing for even nucleation. Moreover, the uniform distribution of N on the layer results in homogeneous zinc ions flux and supports consistent zinc plating while inhibiting dendrites generation. As a result of this unique artificial bi-functional layer, symmetric Zn cells can survive 2500 hours at 2.5 mA cm−2. High-areal-capacity zinc||activated carbon hybrid supercapacitors also demonstrate 20000 cycles at high Coulombic efficiency, thus highlighting the utter convenience and potential of this strategy for modifying rechargeable metal hybrid supercapacitor surfaces." @default.
- W4383888081 created "2023-07-12" @default.
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- W4383888081 date "2023-12-01" @default.
- W4383888081 modified "2023-10-04" @default.
- W4383888081 title "Artificial bi-functional layers promoting Zn2+ desolvation and homogeneous deposition for reversible zinc metal anodes" @default.
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- W4383888081 doi "https://doi.org/10.1016/j.jcis.2023.07.063" @default.
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