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• W4383896264 abstract "Sulfidation of zerovalent iron (SZVI) can strengthen the decontamination ability by promoting the electron transfer from inner Fe0 to external pollutants by iron sulfide (FeSx). Although FeSx forms easily, the mechanism for the FeSx bonding on the ZVI surface through a liquid precipitation method is elusive. In this work, we demonstrate a key pathway for the sulfidation of ZVI, namely, the in situ formation of FeSx on ZVI surface, which leads to chemical bonding across two domains: the pristine ZVI and the newly formed FeSx phase. The two chemically bridged heterophases display superior activity in electron transportation compared to the physically coated SZVI, eventually bringing about the better performance in reducing Cr(VI) species. It is revealed that the formation of chemically bonded FeSx requires balancing the rates for the two processes of Fe(II) release and sulfidation, which can be achieved by tuning the pH and S(-II) concentration. This study elucidates a mechanism for surface generation of FeSx on ZVI, and it provides new perspectives to design high-quality SZVI for environmental applications." @default.
• W4383896264 created "2023-07-12" @default.
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• W4383896264 date "2023-07-11" @default.
• W4383896264 modified "2023-10-09" @default.
• W4383896264 title "Chemical Bond Bridging across Two Domains: Generation of Fe(II) and In Situ Formation of FeS_<i>x</i> on Zerovalent Iron" @default.
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• W4383896264 doi "https://doi.org/10.1021/acs.est.3c02768" @default.
• W4383896264 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37433023" @default.
• W4383896264 hasPublicationYear "2023" @default.
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