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• W4383896454 endingPage "34991" @default.
• W4383896454 startingPage "34983" @default.
• W4383896454 abstract "There is an increasing need for sustainable energy storage solutions as fossil fuels are replaced by renewable energy sources. Multivalent batteries, specifically Mg batteries, are one energy storage technology that researchers continue to develop with hopes to surpass the performance of Li-ion batteries. However, the limited energy density and transport properties of Mg cathodes remain critical challenges preventing the realization of high-performance multivalent batteries. In this work, ABO4 zircon materials (A = Y, Eu and B = V, Cr) are computationally and experimentally evaluated as Mg intercalation cathodes. Remarkably good Mg-ion transport properties were predicted and Mg-ion intercalation was experimentally verified in sol–gel synthesized zircon YVO4, EuVO4, and EuCrO4. Among them, EuVO4 exhibited the best electrochemical performance and demonstrated repeated reversible cycling. While we believe that the one-dimensional diffusion channels and redox-active species tetragonal coordination limit the value of many zircons as high-performance cathodes, their unique structural motif of overlapping polyhedra along the diffusion pathway appears instrumental for promoting good Mg-ion mobility. The motif results in a favorable “6-5-4” change in coordination that avoids unfavorable sites with lower coordination along the diffusion pathway and a structural design metric for future Mg cathode development." @default.
• W4383896454 created "2023-07-12" @default.
• W4383896454 creator A5014983956 @default.
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• W4383896454 date "2023-07-11" @default.
• W4383896454 modified "2023-09-27" @default.
• W4383896454 title "Novel Structural Motif To Promote Mg-Ion Mobility: Investigating ABO₄ Zircons as Magnesium Intercalation Cathodes" @default.
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• W4383896454 doi "https://doi.org/10.1021/acsami.3c05964" @default.
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• W4383896454 hasPublicationYear "2023" @default.
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