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• W4384071498 abstract "Reminiscent to nature’s NAD+/NADH hydride storage and transfer system, we demonstrate here that an iridium complex containing a pyridinium ligand, IrPYE+, is capable of reversibly storing a hydride upon reaction with formate. The hydride in IrPYEH is stable toward air and water, yet it is released in the presence of electrophiles such as acids or carbonyl compounds. The full reversibility of the hydride storage provides access to the hydrogenation procedure that is catalytic in IrPYEH, reaching up to 100,000 turnover numbers and surpassing other related catalysts by several orders of magnitude. With deuterated formate, IrPYED allows for selective deuterium isotope labeling without notable scrambling even in the presence of acids, air, and moisture." @default.
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• W4384071498 date "2023-07-12" @default.
• W4384071498 modified "2023-09-25" @default.
• W4384071498 title "NADH-Type Hydride Storage and Release on a Functional Ligand for Efficient and Selective Hydrogenation Catalysis" @default.
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• W4384071498 doi "https://doi.org/10.1021/acscatal.3c02343" @default.
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