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• W4384077993 endingPage "21070" @default.
• W4384077993 startingPage "21063" @default.
• W4384077993 abstract "The lignin oil produced by rapid pyrolysis of lignin is considered a promising liquid fuel source. Hydrodeoxygenation (HDO) is a kind of efficient method to upgrade the lignin oil, and a high-performance catalyst is key to the hydrodeoxygenation of lignin oil. In this study, a high dispersion and small size Ru nanoparticle loaded N-doped carbon catalyst was derived by the direct pyrolysis of a mixture of ruthenium trichloride and melamine, and it could efficiently convert lignin oil. The lignin oil was completely transformed at 240 °C and 1 MPa H2, and 36.58% cyclohexane was obtained. The formation, surface area, and nitrogen species of the catalyst could be controlled by changing the precursor of the nitrogen-doped carbon support. The percentage of pyridine nitrogen possessed with melamine as a nitrogen-carbon precursor (31.35%) was much higher than that with urea (16.47%) and dicyandiamide (8.20%) as nitrogen-carbon precursors. The presence of pyridine nitrogen could not only serve as the coordination site for even dispersity and stability of Ru nanoparticles but also regulated the electron density of Ru nanoparticles (NPs) and increased the active site Ru0 through electron transfer." @default.
• W4384077993 created "2023-07-13" @default.
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• W4384077993 date "2023-01-01" @default.
• W4384077993 modified "2023-10-16" @default.
• W4384077993 title "Preparation of Ru/N-doped carbon catalysts by induction of different nitrogen source precursors for the hydroprocessing of lignin oil" @default.
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• W4384077993 doi "https://doi.org/10.1039/d3ra01866k" @default.
• W4384077993 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37448633" @default.
• W4384077993 hasPublicationYear "2023" @default.
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