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- W4384155187 abstract "Abstract Developing more extensive methods to understand the underlying structure-property relationship of mechanochromic luminescent molecules is demanding but remains challenging. Herein, the effect of host-guest interaction on the mechanochromic properties of organic molecules is illustrated. A series of pyridinium-functionalized triphenylamine derivatives show bathochromic-shifted emission upon mechanical stimulation. These derivatives bind to cucurbit[8]uril to form homoternary host-guest inclusion complexes through host-stabilized intermolecular charge transfer interactions. Remarkably, the homoternary complexes exhibit longer emission than that of free guests in the solid state (even longer than ground guests), and a further bathochromic-shifted emission is observed upon grinding. Additionally, a heteroternary complex constructed through the encapsulation of pyrene (donor) and pyridinium (acceptor) guest pair in cucurbit[8]uril also displays the mechanochromic luminescent property. This work not only discloses the effect of host-guest inclusion on the mechanochromic property of organic molecules, but also provides a principle and a facile way to design the sequentially red-shifted mechanochromic materials." @default.
- W4384155187 created "2023-07-14" @default.
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- W4384155187 date "2023-07-13" @default.
- W4384155187 modified "2023-10-15" @default.
- W4384155187 title "The host–guest inclusion driven by host-stabilized charge transfer for construction of sequentially red-shifted mechanochromic system" @default.
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- W4384155187 doi "https://doi.org/10.1038/s41467-023-39956-7" @default.
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