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• W4384156233 abstract "Abstract The interaction of a number of gold(III) complexes: Au(phen)X 2 + , Au(bipy)X 2 + (X=Cl, OH, phen=1,10‐phenanthroline, bipy=2,2’‐bipyridile), Au(en) 2 3+ and Au(dien)Cl 2+ with anions of thiol‐containing acids (thiomalate, cysteine and glutathione) in an aqueous solution at pH 2.0 and 7.4, C NaCl =0.2 M was studied. In all cases, the products of gold(III) reduction were highly stable gold(I) thiolate complexes: polymeric Au m (RS) n or monomeric Au(RS) 2 , depending on the conditions. For bipy and phen complexes, the processes were fast and usually completed in less than 1 minute. For the complex with dien, the stage of inner‐sphere reduction was the slowest among the complexes under consideration. For this complex, at pH 7.4 and with a large excess of glutathione, the formation of a relatively long‐lived gold(III) complex was observed, which, according to MS data, has the composition Au(GSH) 4 5– . At ordinary temperature, it decomposes by about 90 % in 20 hours. For other thiols, similar complexes are also formed, but the rate of their decomposition is about 10 times higher." @default.
• W4384156233 created "2023-07-14" @default.
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• W4384156233 date "2023-07-13" @default.
• W4384156233 modified "2023-09-25" @default.
• W4384156233 title "On Redox Processes of Gold(III) Complexes with Biologically Important Thiols: Cysteine, Glutathione, Thiomalate" @default.
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• W4384156233 doi "https://doi.org/10.1002/slct.202301337" @default.
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