Matches in SemOpenAlex for { <https://semopenalex.org/work/W4384157419> ?p ?o ?g. }
- W4384157419 endingPage "144717" @default.
- W4384157419 startingPage "144717" @default.
- W4384157419 abstract "Heavy metal complexes pose a challenge in terms of their resistance to removal due to their stable and intricate structure. In this study, we explored the utilization of Fe and N co-doped biochar derived from rice husk (Fe-N-RHBC) as catalytic particle electrodes in a three-dimensional electro-Fenton (3D-EF) system for the decomplexation and removal of a model pollutant, Ni-EDTA. The characterization analysis and comparison of catalytic activities confirmed the beneficial effects of Fe and N co-doping on various aspects, such as the types of active sites, interfacial electron transfer properties, and H2O2 decomposition capacity. Compared to other investigated oxidation systems, the 3D-EF process demonstrated rapid removal of Ni-EDTA within the initial minute, with a maximum H2O2 utilization of 99.1% after 30 min. The prepared catalytic particle electrodes exhibited high stability and catalytic capacity even after three consecutive cycles. Throughout the reaction, several processes, including anode oxidation, particle electrode polarization, catalysis, and adsorption of Fe-N-RHBC, as well as cathodic electro-deposition, synergistically contributed to the treatment of Ni-EDTA. The surface-bound O2•− radicals and 1O2 generated by the Fe-N-RHBC catalytic particle electrode played a crucial role in the decomplexation and removal of Ni-EDTA. Building upon these findings, we further proposed potential mechanisms for the removal of Ni-EDTA in the 3D-EF system using the Fe-N-RHBC catalytic particle electrode." @default.
- W4384157419 created "2023-07-14" @default.
- W4384157419 creator A5019376351 @default.
- W4384157419 creator A5033013991 @default.
- W4384157419 creator A5050989699 @default.
- W4384157419 creator A5057049857 @default.
- W4384157419 creator A5058560666 @default.
- W4384157419 creator A5072081832 @default.
- W4384157419 creator A5079110296 @default.
- W4384157419 date "2023-09-01" @default.
- W4384157419 modified "2023-09-27" @default.
- W4384157419 title "Enhanced removal of Ni-EDTA by three-dimensional electro-Fenton process using Fe-N-doped biochar as catalytic particle electrodes" @default.
- W4384157419 cites W1971296006 @default.
- W4384157419 cites W1975921755 @default.
- W4384157419 cites W1988923205 @default.
- W4384157419 cites W2002246323 @default.
- W4384157419 cites W2026773165 @default.
- W4384157419 cites W2044205613 @default.
- W4384157419 cites W2056718604 @default.
- W4384157419 cites W2065630329 @default.
- W4384157419 cites W2083651101 @default.
- W4384157419 cites W2127011617 @default.
- W4384157419 cites W2171128235 @default.
- W4384157419 cites W2399065299 @default.
- W4384157419 cites W2576257030 @default.
- W4384157419 cites W2591048484 @default.
- W4384157419 cites W2593454506 @default.
- W4384157419 cites W2639656676 @default.
- W4384157419 cites W2738858711 @default.
- W4384157419 cites W2766554498 @default.
- W4384157419 cites W2793226524 @default.
- W4384157419 cites W2802615836 @default.
- W4384157419 cites W2806677203 @default.
- W4384157419 cites W2883583069 @default.
- W4384157419 cites W2885002054 @default.
- W4384157419 cites W2889529087 @default.
- W4384157419 cites W2895209668 @default.
- W4384157419 cites W2895304269 @default.
- W4384157419 cites W2908556609 @default.
- W4384157419 cites W2913038549 @default.
- W4384157419 cites W2920930698 @default.
- W4384157419 cites W2921410295 @default.
- W4384157419 cites W2933649394 @default.
- W4384157419 cites W2938552892 @default.
- W4384157419 cites W2946055735 @default.
- W4384157419 cites W2947351355 @default.
- W4384157419 cites W2969636361 @default.
- W4384157419 cites W2972654400 @default.
- W4384157419 cites W2994720660 @default.
- W4384157419 cites W3015589213 @default.
- W4384157419 cites W3025336171 @default.
- W4384157419 cites W3029851150 @default.
- W4384157419 cites W3035417573 @default.
- W4384157419 cites W3046343005 @default.
- W4384157419 cites W3066861833 @default.
- W4384157419 cites W3089650045 @default.
- W4384157419 cites W3090116547 @default.
- W4384157419 cites W3097963502 @default.
- W4384157419 cites W3116043432 @default.
- W4384157419 cites W3123775168 @default.
- W4384157419 cites W3131772070 @default.
- W4384157419 cites W3132081696 @default.
- W4384157419 cites W3159533393 @default.
- W4384157419 cites W3164702838 @default.
- W4384157419 cites W3195126238 @default.
- W4384157419 cites W3195743195 @default.
- W4384157419 cites W3197050481 @default.
- W4384157419 cites W3204875577 @default.
- W4384157419 cites W3207544205 @default.
- W4384157419 cites W3217349302 @default.
- W4384157419 cites W4205400499 @default.
- W4384157419 cites W4206649148 @default.
- W4384157419 cites W4220720604 @default.
- W4384157419 cites W4220789302 @default.
- W4384157419 cites W4220844122 @default.
- W4384157419 cites W4221018172 @default.
- W4384157419 cites W4280597028 @default.
- W4384157419 cites W4282000003 @default.
- W4384157419 cites W4289443675 @default.
- W4384157419 cites W4289596365 @default.
- W4384157419 cites W4295015403 @default.
- W4384157419 cites W4297828448 @default.
- W4384157419 cites W4309340883 @default.
- W4384157419 cites W4312193258 @default.
- W4384157419 doi "https://doi.org/10.1016/j.cej.2023.144717" @default.
- W4384157419 hasPublicationYear "2023" @default.
- W4384157419 type Work @default.
- W4384157419 citedByCount "0" @default.
- W4384157419 crossrefType "journal-article" @default.
- W4384157419 hasAuthorship W4384157419A5019376351 @default.
- W4384157419 hasAuthorship W4384157419A5033013991 @default.
- W4384157419 hasAuthorship W4384157419A5050989699 @default.
- W4384157419 hasAuthorship W4384157419A5057049857 @default.
- W4384157419 hasAuthorship W4384157419A5058560666 @default.
- W4384157419 hasAuthorship W4384157419A5072081832 @default.
- W4384157419 hasAuthorship W4384157419A5079110296 @default.
- W4384157419 hasConcept C111368507 @default.
- W4384157419 hasConcept C127313418 @default.