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- W4384204772 abstract "The separation of photogenerated charges is vital for photocatalysis. Here, we report a wireless photoelectrochemical strategy for efficient charge separation on an optoelectronic synergy-driven nanoparticulate semiconductor. Using g-C3N4/Fe–TiO2 as model semiconductor nanoparticles, an advanced oxidation process (AOP) for water remediation was established with the activity and O2•– photogeneration quantum efficiency being significantly improved (i.e., 9.7 times compared to conventional photoelectrocatalysis and 5.9 times that of photocatalysis, respectively). More importantly, this strategy has a wide range of applications for the removal of different refractory organic pollutants with a strong tolerance for a supporting electrolyte. The extraordinary catalytic performance was attributed to a synergistic effect between photochemistry and electrochemistry on the particle surface, where numerous nanobipolar electrodes were generated under an electric field to trigger the reduction of electrogenerated O2 to form reactive oxygen species. This work provides a promising AOP strategy of a photoelectrochemical-driven nanoparticulate semiconductor for challenging water remediation." @default.
- W4384204772 created "2023-07-14" @default.
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- W4384204772 date "2023-07-13" @default.
- W4384204772 modified "2023-09-25" @default.
- W4384204772 title "Wireless Photoelectrochemical Strategy Driven by Nanobipolar Electrodes for Water Remediation" @default.
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- W4384204772 doi "https://doi.org/10.1021/acsestwater.3c00101" @default.
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