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• W4384206965 endingPage "144768" @default.
• W4384206965 startingPage "144768" @default.
• W4384206965 abstract "The need to decrease environmental pollution, reduce energy consumption and produce high-purity chemicals has become an increasingly important driving force for sulfur dioxide (SO2) capture. The efficient capture of low concentrations of SO2, a highly corrosive acid gas that is not typically present in high concentrations in industrial settings, is a major challenge. Herein, a novel phosphate-functionalized metal–organic framework, ZU-801, is designed with precisely controlled pore sizes and chemical environment to achieve excellent adsorption capacity for SO2 (1.44 mmol g−1 at 0.002 bar, 2.00 mmol g−1 at 0.01 bar) and high IAST selectivities for SO2/CO2 (1 4 5), which provides great potential for selective capture of SO2. ZU-801 shows excellent stability to air, water, SO2, strong acid and strong base solutions, and it is thermally stable up to 733 K. Additionally, ZU-801 exhibits outstanding separation ability in removing SO2 from SO2/CO2 mixtures at temperatures as high as 383 K or in humid environments. This work demonstrates the potential of designing ion-functionalized ultramicroporous materials with tailored pore sizes and porous chemical environments for efficient capture and separation of SO2 and sheds light on designing stable high-performance materials that operate at high temperatures." @default.
• W4384206965 created "2023-07-14" @default.
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• W4384206965 date "2023-09-01" @default.
• W4384206965 modified "2023-10-15" @default.
• W4384206965 title "A novel robust phosphate-functionalized metal–organic framework for deep desulfurization at wide temperature" @default.
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• W4384206965 doi "https://doi.org/10.1016/j.cej.2023.144768" @default.
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