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- W4384207948 abstract "Nanomaterials are widely used in constructing reverse electrodialysis (RED) systems with charged nanochannels for osmotic energy harvesting. However, preparing low-cost, large-scale, and high-performance RED systems with significantly improved ion selectivity, ion flux, and output power density is still a challenge. Herein, we develop a facile solution-casting method to fabricate oriented regenerated cellulose (RC)/carbon nanotubes (CNTs) nanohybrid membranes. After integrating chemical modification (i.e., TEMPO oxidation and quaternization) and structural densification, both negatively charged N-RC/N-CNTs and positively charged P-RC/P-CNTs membranes demonstrated significantly enhanced ionic conductivity in a low-concentration solution (4.02×10−4 and 3.59×10−4 S cm−1, respectively). Particularly, the P–N unit not only yields an output power density of 5.28 W m−2 in a 50-fold concentration gradient, which exceeds the commercial standard (5 W m−2), but also achieves long-term stability over 50 days. As a proof of concept, we created a RED system with 20 P–N units connected in series which successfully powered an electronic calculator with an output voltage of 2.06 V under artificial seawater and river water conditions. This work improves the development of natural renewable materials for high-performance osmotic energy conversion." @default.
- W4384207948 created "2023-07-14" @default.
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- W4384207948 date "2023-10-01" @default.
- W4384207948 modified "2023-10-16" @default.
- W4384207948 title "Scalable fabrication of regenerated cellulose nanohybrid membranes integrating opposite charges and aligned nanochannels for continuous osmotic energy harvesting" @default.
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- W4384207948 doi "https://doi.org/10.1016/j.nanoen.2023.108693" @default.
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