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- W4384284766 abstract "Ladder-type structures can impart exceptional stability to polymeric electronic materials. This article introduces a new class of conductive polymers featuring a fully ladder-type backbone. A judicious molecular design strategy enables the synthesis of a low-defect ladder polymer, which can be efficiently oxidized and acid-doped to achieve its conductive state. The structural elucidation of this polymer and the characterization of its open-shell nature are facilitated with the assistance of studies on small molecular models. An autonomous robotic system is used to optimize the conductivity of the polymer thin film, achieving over 7 mS cm-1. Impressively, this polymer demonstrates unparalleled stability in strong acid and under harsh UV-irradiation, significantly surpassing commercial benchmarks like PEDOT:PSS and polyaniline. Moreover, it displays superior durability across numerous redox cycles as the active material in an electrochromic device and as the pseudocapacitive material in a supercapacitor device. This work provides structural design guidance for durable conductive polymers for long-term device operation." @default.
- W4384284766 created "2023-07-15" @default.
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- W4384284766 date "2023-01-01" @default.
- W4384284766 modified "2023-10-18" @default.
- W4384284766 title "Synthesis and exceptional operational durability of polyaniline-inspired conductive ladder polymers" @default.
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- W4384284766 doi "https://doi.org/10.1039/d3mh00883e" @default.
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