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- W4384343843 abstract "Abstract Palladium (Pd) shows high activity in a variety of catalysis reactions that refer to the activation of the carbon-halogenation bond, and single-atom Pd catalysts have received significant attention as new technology. Nevertheless, there is a huge knowledge gap regarding which Pd sites could form highly reactive centers. It is unclear whether single-atom Pd sites are active in this process or not. In this study, we synthesized Pd/TiO2 nanosheets with Pd loadings of 1%, 5%, and 10% and designed single atom Pd sites and Pd nanoparticles on similar substrates. A scanning transmission electron microscope was used to characterize the synthesized Pd catalysts. As a catalyst, Pd/TiO2 featuring Pd NPs showed high activity in activating the carbon-halogen bond in the activation of carbon-chloride bond, whereas Pd/TiO2 with single Pd atoms showed very low activity in this pros. Accordingly, our results demonstrate that the activation of carbon-halogen bonds cannot be catalyzed by the single-atom Pd sites and emphasize the significance of the ensemble effect in determining the activity of Pd sites." @default.
- W4384343843 created "2023-07-15" @default.
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- W4384343843 date "2023-07-01" @default.
- W4384343843 modified "2023-09-23" @default.
- W4384343843 title "Insight into the Effects of Pd Single-atom Particles in the Activation of the Carbon-Chloride Bond" @default.
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- W4384343843 doi "https://doi.org/10.1088/1742-6596/2539/1/012080" @default.
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