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• W4384405907 abstract "Abstract The electrochemical reduction of CO 2 to produce sustainable fuels and chemicals has attracted great attention in recent years. It is shown that surface‐modified carbons catalyze the CO 2 RR. This study reports a strategy to modify the surface of commercially available carbon materials by adding oxygen and nitrogen surface groups without modifying its graphitic structure. Clear differences in CO 2 RR activity, selectivity and the turnover frequency between the surface‐modified carbons were observed, and these differences were ascribed to the nature of the surface groups chemistry and the point of zero charge (PZC). The results show that nitrogen‐containing surface groups are highly selective towards the formation of CO from the electroreduction of CO 2 in comparison with the oxygen‐containing surface groups, and the carbon without surface groups. This demonstrates that the selectivity of carbon for CO 2 RR can be rationally tuned by simply altering the surface chemistry via surface functionalization." @default.
• W4384405907 created "2023-07-16" @default.
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• W4384405907 date "2023-08-08" @default.
• W4384405907 modified "2023-10-14" @default.
• W4384405907 title "Surface‐Modified Carbon Materials for CO₂ Electroreduction" @default.
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• W4384405907 doi "https://doi.org/10.1002/ejic.202300152" @default.
• W4384405907 hasPublicationYear "2023" @default.
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