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• W4384406555 abstract "Layered ammonium vanadate materials exhibit significant mass-specific capacity and ion transport rate due to their small molecular weight and large ionic radius. However, the strong electrostatic interactions of Zn2+ and V–O bonds and the fragile ionic bonding of N-H…O bonds hinder their development. Therefore, this work reports Mg2+ doping NH4V4O10 materials accompanied by flower-like morphology to lower the migration energy barrier and inhibit amine dissolution. Owing to the 3D-flower-like morphology and the combined impact of Mg2+ and structural water, the binding of Zn2+…V-O is significantly enhanced and additional ion channels were constructed. Pre-intercalated Mg2+ enhances the structural integrity and prevents irreversible deammoniation from obtaining excellent cyclic stability. Density functional theory (DFT) calculations show that MNVO provides a smoother Zn2+ diffusion path with a lower migration barrier. Benefited from these advantages, the MNVO cathode exhibits a high specific capacity of 410 mAh g−1 at 0.1 A g−1, satisfactory cyclic stability (90.2 % capacity retention at 10 A g−1 after 5000 cycles), and capable rate ability (118 mAh g−1 at 25 A g−1) within 0.4-1.5 V. Furthermore, the zinc ion storage mechanism in the MNVO cathode is investigated through multiple analyses." @default.
• W4384406555 created "2023-07-16" @default.
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• W4384406555 date "2023-07-14" @default.
• W4384406555 modified "2023-10-17" @default.
• W4384406555 title "Magnesium Ion Doping and Micro‐Structural Engineering Assist NH₄V₄O₁₀ as a High‐Performance Aqueous Zinc Ion Battery Cathode" @default.
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• W4384406555 doi "https://doi.org/10.1002/adfm.202306205" @default.
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