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• W4384497742 abstract "Doped CaZnOS materials show great potential for mechanoluminescence (ML) applications spanning the ultraviolet-visible-near infrared (UV–vis–NIR) range. However, conflicting reports regarding the generation and reproducibility of ML hinder the understanding and practical utilization of these materials. To address this issue, a comprehensive characterization strategy combining NIR laser-assisted de-trapping, UV irradiation-induced trap-filling, in situ mechanical stimulation, and continuous ML recording is proposed. Herein, the ML behaviors of four representative doped CaZnOS materials (Mn2+, Bi3+, Er3+, and Ce3+) are investigated using this approach. The results reveal that de-trapped materials exhibit non-trap-controlled ML, wherein ML intensity gradually weakens under successive mechanical stimuli without self-recovery. In contrast, trap-filled materials demonstrate both trap-controlled ML and non-trap-controlled ML, with the former predominantly contributing to the overall ML intensity. Notably, trap-controlled ML shows only partial recovery after trap filling. The non-trap-controlled ML is attributed to plastic ML and destructive ML phenomena, while explaining trap-controlled ML through the carrier de-trapping model. These results not only clarify conflicting reports but also provide clear insights into the ML properties and mechanisms of CaZnOS-based materials, facilitating advancements in practical applications. Furthermore, the developed characterization strategy is expected to serve as a valuable reference for establishing standardized protocols to evaluate ML performance." @default.
• W4384497742 created "2023-07-18" @default.
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• W4384497742 date "2023-07-17" @default.
• W4384497742 modified "2023-09-27" @default.
• W4384497742 title "Unraveling Mechanoluminescent Mechanisms in Doped CaZnOS Materials: Co‐Mediation of Trap‐Controlled and Non‐Trap‐Controlled Processes" @default.
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• W4384497742 doi "https://doi.org/10.1002/adfm.202305482" @default.
• W4384497742 hasPublicationYear "2023" @default.
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