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- W4384639687 abstract "Abstract UO 2 F 2 abstracts F − anions from TlF in liquid ammonia solution and the compound [Tl 2 (NH 3 ) 6 ][{UO 2 F 2 (NH 3 )} 2 (μ‐F) 2 ] is formed. The compound has been characterized by single crystal X‐ray diffraction, Raman spectroscopy and quantum‐chemical calculations for the solid state. Quantum‐chemical investigation of the [{UO 2 F 2 (NH 3 )} 2 (μ‐F) 2 ] 2− anion showed that the U−(μ‐F)−U σ‐3c‐4e‐bond is essentially ionic. The [Tl 2 (NH 3 ) 6 ] 2+ cation shows a thallophilic Tl⋅⋅⋅Tl interaction. Fluoride ion affinities (FIAs) were calculated for different UO 2 2+ species [UO 2 F x ] 2− x and [UO 2 F x (NH 3 ) 5 −x ] 2− x with x =0 to 4." @default.
- W4384639687 created "2023-07-19" @default.
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- W4384639687 date "2023-08-01" @default.
- W4384639687 modified "2023-10-14" @default.
- W4384639687 title "A Dinuclear Uranium Complex [{UO2F2(NH3)}2(μ‐F)2]2– from Reaction of TlF and UO2F2 in anhydrous Ammonia and Fluoride Ion Affinities for some Uranyl(VI) Species [UO2F x ]2–xand [UO2F x (NH3)5–x]2–x" @default.
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- W4384639687 doi "https://doi.org/10.1002/ejic.202300387" @default.
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