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• W4384662826 abstract "Epitaxial cathodes in lithium-ion microbatteries are ideal model systems to understand mass and charge transfer across interfaces, plus interphase degradation processes during cycling. Importantly, if grown at <450 °C, they also offer potential for complementary metal-oxide-semiconductor (CMOS) compatible microbatteries for the Internet of Things, flexible electronics, and MedTech devices. Currently, prominent epitaxial cathodes are grown at high temperatures (>600 °C), which imposes both manufacturing and scale-up challenges. Herein, we report structural and electrochemical studies of epitaxial LiMn2O4 (LMO) thin films grown on a new current collector material, NiCo2O4 (NCO). We achieve this at the low temperature of 360 °C, ∼200 °C lower than existing current collectors SrRuO3 and LaNiO3. Our films achieve a discharge capacity of >100 mAh g-1 for ∼6000 cycles with distinct LMO redox signatures, demonstrating long-term electrochemical stability of our NCO current collector. Hence, we show a route toward high-performance microbatteries for a range of miniaturized electronic devices." @default.
• W4384662826 created "2023-07-20" @default.
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• W4384662826 date "2023-07-18" @default.
• W4384662826 modified "2023-10-14" @default.
• W4384662826 title "Low Temperature Epitaxial LiMn₂O₄ Cathodes Enabled by NiCo₂O₄ Current Collector for High-Performance Microbatteries" @default.
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• W4384662826 doi "https://doi.org/10.1021/acsenergylett.3c01094" @default.
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• W4384662826 hasPublicationYear "2023" @default.
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