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- W4384700564 abstract "The structures of the adsorbed water molecules in AlPO4–5, their structural evolutions and changes of Al-O-P angles between tetrahedra upon water adsorption were investigated by infrared spectroscopy. The results indicate that Al-H2O coordination is present in the channels and the adsorbed water molecules are in low, intermediate and strong hydrogen-bonded environments. The population of the water species varies with a sudden enhancement from 70–140 min, showing similarity to the reported abnormal isotherm due to the increase of host-guest interaction sites. This large-scale uptake of water accelerates structural transformations of water from intermediate to strong hydrogen-bonded structures. Moreover, the water-framework interaction facilitates the closure of Al-O-P angles and thus results in the framework contraction. This study opens the door to a good knowledge of the hydrogen-bonded structures of H2O and framework deformation in hydrated AlPO4–5 from the viewpoint of infrared spectroscopy." @default.
- W4384700564 created "2023-07-20" @default.
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- W4384700564 date "2023-11-01" @default.
- W4384700564 modified "2023-10-16" @default.
- W4384700564 title "Water adsorption and framework evolution in AlPO4-5: an infrared spectroscopic study" @default.
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- W4384700564 doi "https://doi.org/10.1016/j.molstruc.2023.136245" @default.
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