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• W4384819428 abstract "Hitherto, it remains a great challenge to stabilize electrolyte-electrode interfaces and impede lithium dendrite proliferation in lithium-metal batteries with high-capacity nickel-rich LiNx Coy Mn1-x-y O2 (NCM) layer cathodes. Herein, a special molecular-level-designed polymer electrolyte is prepared by the copolymerization of hexafluorobutyl acrylate and methylene bisacrylamide to construct dual-reinforced stable interfaces. Verified by X-ray photoelectron spectroscopy depth profiling, there are favorable solid electrolyte interphase (SEI) layers on Li metal anodes and robust cathode electrolyte interphase (CEI) on Ni-rich cathodes. The SEI enriched in lithiophilic N-(C)3 guides the homogenous distribution of Li+ and facilitates the transport of Li+ through LiF and Li3 N, promoting uniform Li+ plating and stripping. Moreover, the CEI with antioxidative amide groups can suppress the parasitic reactions between cathode and electrolyte and the structural degradation of cathode. Meanwhile, a unique two-stage rheology-tuning UV polymerization strategy is utilized, which is quite suited for continuous electrolyte fabrication with environmental friendliness. The fabricated polymer electrolyte exhibits a high ionic conductivity of 1.01 mS cm-1 at room temperature. 4.5 V NCM622//Li batteries achieve prolonged operation with a retention rate of 85.0% after 500 cycles at 0.5 C. This work provides new insights into molecular design and processibility design for polymer-based high-voltage batteries." @default.
• W4384819428 created "2023-07-21" @default.
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• W4384819428 date "2023-10-09" @default.
• W4384819428 modified "2023-10-18" @default.
• W4384819428 title "Enabling Scalable Polymer Electrolyte with Dual‐Reinforced Stable Interface for 4.5 V Lithium Metal Batteries" @default.
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• W4384819428 doi "https://doi.org/10.1002/adma.202304951" @default.
• W4384819428 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37467170" @default.
• W4384819428 hasPublicationYear "2023" @default.
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