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- W4384926086 abstract "Photon avalanching nanoparticles (ANPs) exhibit extremely nonlinear upconverted emission valuable for sub-diffraction imaging, nanoscale sensing, and optical computing. Avalanching has been demonstrated with Tm3+, Nd3+ or Pr3+-doped nanocrystals, but their emission is limited to 600 and 800 nm, restricting applications. Here, we utilize Gd3+-assisted energy migration to tune the emission wavelengths of Tm3+-sensitized ANPs and generate highly nonlinear emission of Eu3+, Tb3+, Ho3+, and Er3+ ions. The upconversion intensities of these spectrally discrete ANPs scale with the nonlinearity factor s = 10-17 under 1064 nm excitation at power densities as low as 6 kW/cm2. This strategy for imprinting avalanche behavior on remote emitters can be extended to fluorophores adjacent to ANPs, as we demonstrate with CdS/CdSe/CdS core/shell/shell quantum dots. ANPs with rationally designed energy transfer networks provide the means to transform conventional linear emitters into a highly nonlinear ones, expanding the use of photon avalanching in biological, chemical, and photonic applications." @default.
- W4384926086 created "2023-07-22" @default.
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- W4384926086 date "2023-07-20" @default.
- W4384926086 modified "2023-10-10" @default.
- W4384926086 title "A Generalized Approach to Photon Avalanche Upconversion in Luminescent Nanocrystals" @default.
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- W4384926086 doi "https://doi.org/10.1021/acs.nanolett.3c01955" @default.
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