Matches in SemOpenAlex for { <https://semopenalex.org/work/W4384927405> ?p ?o ?g. }
Showing items 1 to 100 of
100
with 100 items per page.
- W4384927405 endingPage "10166" @default.
- W4384927405 startingPage "10161" @default.
- W4384927405 abstract "Methane pyrolysis is a unique approach toward generating hydrogen and valuable carbon products, with the added advantage of low to near-zero CO2 emissions. Currently, the most popular method for hydrogen production is steam methane reforming, which generates more than 10 kg of CO2 for every 1 kg of hydrogen. By comparison, methane pyrolysis produces hydrogen and solid carbon with no COx biproduct. Methane pyrolysis on a conventional solid catalyst exhibits low activation energy, but the carbon coproduct cannot be separated and rapidly poisons the surface (coking). On the other hand, molten liquid metal catalysts have been shown to have the advantage of separatable carbon, but their high activation energy limits the rate of the reaction and potential for economic industrialization. In this work, methane pyrolysis was shown using a multiphase molten metal reactor where both liquid and solid metal alloy catalysts were in equilibrium. Catalytic measurements using a Sn–Ni melt showed that operating the reactor in the two-phase region of the Sn–Ni phase diagram decreased the apparent activation energy from 355 kJ/mol in the liquid-only melt to 158 kJ/mol, all while maintaining the ability to separate and recover graphitic carbon." @default.
- W4384927405 created "2023-07-22" @default.
- W4384927405 creator A5006475296 @default.
- W4384927405 creator A5084050529 @default.
- W4384927405 date "2023-07-20" @default.
- W4384927405 modified "2023-09-24" @default.
- W4384927405 title "Methane Pyrolysis Using a Multiphase Molten Metal Reactor" @default.
- W4384927405 cites W1982597676 @default.
- W4384927405 cites W2021178489 @default.
- W4384927405 cites W2025785539 @default.
- W4384927405 cites W2050684431 @default.
- W4384927405 cites W2065030601 @default.
- W4384927405 cites W2071228067 @default.
- W4384927405 cites W2088497526 @default.
- W4384927405 cites W2135580922 @default.
- W4384927405 cites W2591042472 @default.
- W4384927405 cites W2594391820 @default.
- W4384927405 cites W2610095455 @default.
- W4384927405 cites W2746479387 @default.
- W4384927405 cites W2769191683 @default.
- W4384927405 cites W2791247647 @default.
- W4384927405 cites W2791497094 @default.
- W4384927405 cites W2836897415 @default.
- W4384927405 cites W2900965041 @default.
- W4384927405 cites W2917844056 @default.
- W4384927405 cites W2968284787 @default.
- W4384927405 cites W2973933198 @default.
- W4384927405 cites W3022002070 @default.
- W4384927405 cites W3032859978 @default.
- W4384927405 cites W3101168194 @default.
- W4384927405 cites W3109029990 @default.
- W4384927405 cites W3128796903 @default.
- W4384927405 cites W3165791150 @default.
- W4384927405 cites W3195350639 @default.
- W4384927405 cites W4206379970 @default.
- W4384927405 cites W4280616963 @default.
- W4384927405 cites W4293740024 @default.
- W4384927405 cites W4306963289 @default.
- W4384927405 cites W4308905277 @default.
- W4384927405 cites W4320713526 @default.
- W4384927405 doi "https://doi.org/10.1021/acscatal.3c02955" @default.
- W4384927405 hasPublicationYear "2023" @default.
- W4384927405 type Work @default.
- W4384927405 citedByCount "0" @default.
- W4384927405 crossrefType "journal-article" @default.
- W4384927405 hasAuthorship W4384927405A5006475296 @default.
- W4384927405 hasAuthorship W4384927405A5084050529 @default.
- W4384927405 hasBestOaLocation W43849274051 @default.
- W4384927405 hasConcept C104779481 @default.
- W4384927405 hasConcept C127413603 @default.
- W4384927405 hasConcept C140205800 @default.
- W4384927405 hasConcept C159985019 @default.
- W4384927405 hasConcept C161790260 @default.
- W4384927405 hasConcept C178790620 @default.
- W4384927405 hasConcept C179104552 @default.
- W4384927405 hasConcept C185592680 @default.
- W4384927405 hasConcept C192562407 @default.
- W4384927405 hasConcept C202189072 @default.
- W4384927405 hasConcept C36759035 @default.
- W4384927405 hasConcept C42360764 @default.
- W4384927405 hasConcept C43535742 @default.
- W4384927405 hasConcept C512968161 @default.
- W4384927405 hasConcept C516920438 @default.
- W4384927405 hasConceptScore W4384927405C104779481 @default.
- W4384927405 hasConceptScore W4384927405C127413603 @default.
- W4384927405 hasConceptScore W4384927405C140205800 @default.
- W4384927405 hasConceptScore W4384927405C159985019 @default.
- W4384927405 hasConceptScore W4384927405C161790260 @default.
- W4384927405 hasConceptScore W4384927405C178790620 @default.
- W4384927405 hasConceptScore W4384927405C179104552 @default.
- W4384927405 hasConceptScore W4384927405C185592680 @default.
- W4384927405 hasConceptScore W4384927405C192562407 @default.
- W4384927405 hasConceptScore W4384927405C202189072 @default.
- W4384927405 hasConceptScore W4384927405C36759035 @default.
- W4384927405 hasConceptScore W4384927405C42360764 @default.
- W4384927405 hasConceptScore W4384927405C43535742 @default.
- W4384927405 hasConceptScore W4384927405C512968161 @default.
- W4384927405 hasConceptScore W4384927405C516920438 @default.
- W4384927405 hasFunder F4320323278 @default.
- W4384927405 hasFunder F4320329497 @default.
- W4384927405 hasIssue "15" @default.
- W4384927405 hasLocation W43849274051 @default.
- W4384927405 hasOpenAccess W4384927405 @default.
- W4384927405 hasPrimaryLocation W43849274051 @default.
- W4384927405 hasRelatedWork W1473694001 @default.
- W4384927405 hasRelatedWork W1971926200 @default.
- W4384927405 hasRelatedWork W2035742040 @default.
- W4384927405 hasRelatedWork W2072056341 @default.
- W4384927405 hasRelatedWork W2082205067 @default.
- W4384927405 hasRelatedWork W2379888826 @default.
- W4384927405 hasRelatedWork W2416637559 @default.
- W4384927405 hasRelatedWork W2905597440 @default.
- W4384927405 hasRelatedWork W3145780616 @default.
- W4384927405 hasRelatedWork W4385789636 @default.
- W4384927405 hasVolume "13" @default.
- W4384927405 isParatext "false" @default.
- W4384927405 isRetracted "false" @default.
- W4384927405 workType "article" @default.