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• W4385232807 abstract "To enhance the progress of hydrate-based technologies, obtaining accurate and comprehensive data on hydrate equilibria is vital. The presence of mineral salts in water necessitates an examination of their impact on the phase behavior of gas hydrates. This research aims to explore the influence of NaCl and MgCl2, the primary dissolved salts in natural water, on the tetrahydrofuran (THF)–CH4 hydrate system. Experiments are conducted using the isochoric pressure search method with a step-heating technique, covering a range of pressures (1–55 MPa), temperatures (283–300 K), and THF mass fractions (0.05–0.19). The Chen and Guo theory is utilized to extend a thermodynamic model that predicts the behavior of the THF–CH4 hydrate system in the absence or presence of mineral salts. The model demonstrates a satisfactory level of consistency with the generated hydrate data, with an average absolute relative deviation of only 6.05%. Methane’s properties in the gas phase are derived using the Soave–Redlich–Kwong equation of state (SRK EoS). Additionally, the e-UNIQUAC model is employed to calculate the activity of water and the activity coefficient of THF in the electrolyte aqueous phase. The experimental results indicate that THF effectively addresses the challenges associated with methane hydrate formation in saline water, making it a promising promoter. Furthermore, the study reveals that the inhibitory effect of salts is more pronounced in concentrated THF solutions, and increasing the pressure for hydrate formation enhances the inhibitory effect of salts." @default.
• W4385232807 created "2023-07-26" @default.
• W4385232807 creator A5077717565 @default.
• W4385232807 creator A5087601087 @default.
• W4385232807 date "2023-07-25" @default.
• W4385232807 modified "2023-10-16" @default.
• W4385232807 title "Effects of Sea Salts on the Phase Behavior and Synthesis of Methane Hydrates + THF: An Experimental and Theoretical Study" @default.
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• W4385232807 doi "https://doi.org/10.1021/acs.iecr.3c00351" @default.
• W4385232807 hasPublicationYear "2023" @default.
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