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- W4385235148 abstract "Abstract Over the past few decades, exciton-polaritons have attracted substantial research interest due to their half-light-half-matter bosonic nature. Coupling exciton-polaritons with magnetic orders grants access to rich many-body phenomena, but has been limited by the availability of material systems that exhibit simultaneous exciton resonances and magnetic ordering. Here we report magnetically-dressed microcavity exciton-polaritons in the van der Waals antiferromagnetic (AFM) semiconductor CrSBr coupled to a Tamm plasmon microcavity. Angle-resolved spectroscopy reveals an exceptionally high exciton-photon coupling strength attaining 169 meV, demonstrating ultrastrong coupling that persists up to room temperature. Temperature-dependent exciton-polariton spectroscopy senses the magnetic order change from AFM to paramagnetic in CrSBr, confirming its magnetic nature. By applying an out-of-plane magnetic field, an effective tuning of the polariton energy is further achieved while maintaining the ultrastrong exciton-photon coupling strength, which is attributed to the spin canting process that modulates the interlayer exciton interaction. Our work proposes a hybrid quantum platform enabled by robust opto-electronic-magnetic coupling, promising for quantum interconnects and transducers." @default.
- W4385235148 created "2023-07-26" @default.
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- W4385235148 date "2023-07-26" @default.
- W4385235148 modified "2023-10-13" @default.
- W4385235148 title "Magnetically-dressed CrSBr exciton-polaritons in ultrastrong coupling regime" @default.
- W4385235148 doi "https://doi.org/10.21203/rs.3.rs-3164083/v1" @default.
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