FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4385442606> ?p ?o ?g. }

• W4385442606 endingPage "16982" @default.
• W4385442606 startingPage "16978" @default.
• W4385442606 abstract "The electrochemical CO2 reduction reaction (eCO2RR) under acidic conditions has become a promising way to achieve high CO2 utilization because of the inhibition of undesirable carbonate formation that typically occurs under neutral and alkaline conditions. Herein, unprecedented and highly active ditin(IV) sites were integrated into the nanopores of a metal–organic framework, namely NU-1000-Sn, by a “ship-in-a-bottle” strategy. NU-1000-Sn delivers nearly 100% formic acid Faradaic efficiency at an industry current density of 260 mA cm–2 with a high single-pass CO2 utilization of 95% in an acidic solution (pH = 1.67). No obvious degradation was observed over 15 hours of continuous operation at the current density of 260 mA cm–2, representing the remarkable eCO2RR performance in acidic electrolyte to date. The mechanism study shows that both oxygen atoms of the key intermediate *HCOO can coordinate to the two adjacent Sn atoms in a ditin(IV) site simultaneously. Such bridging coordination is conducive to the hydrogenation of CO2, thus leading to high performance." @default.
• W4385442606 created "2023-08-02" @default.
• W4385442606 creator A5012950953 @default.
• W4385442606 creator A5014586466 @default.
• W4385442606 creator A5032221523 @default.
• W4385442606 creator A5064527448 @default.
• W4385442606 date "2023-08-01" @default.
• W4385442606 modified "2023-10-15" @default.
• W4385442606 title "“Ship-in-a-Bottle” Integration of Ditin(IV) Sites into a Metal–Organic Framework for Boosting Electroreduction of CO₂ in Acidic Electrolyte" @default.
• W4385442606 cites W2007082361 @default.
• W4385442606 cites W2025831662 @default.
• W4385442606 cites W2063116381 @default.
• W4385442606 cites W2560545729 @default.
• W4385442606 cites W2780453684 @default.
• W4385442606 cites W2792748777 @default.
• W4385442606 cites W2885627064 @default.
• W4385442606 cites W2888234541 @default.
• W4385442606 cites W2897605246 @default.
• W4385442606 cites W2904352928 @default.
• W4385442606 cites W2953552015 @default.
• W4385442606 cites W2999656933 @default.
• W4385442606 cites W3107960248 @default.
• W4385442606 cites W3116535123 @default.
• W4385442606 cites W3118899616 @default.
• W4385442606 cites W3120711935 @default.
• W4385442606 cites W3129738768 @default.
• W4385442606 cites W3137414459 @default.
• W4385442606 cites W3137759449 @default.
• W4385442606 cites W3159856869 @default.
• W4385442606 cites W3165555416 @default.
• W4385442606 cites W3175247671 @default.
• W4385442606 cites W3181081593 @default.
• W4385442606 cites W3183385567 @default.
• W4385442606 cites W3185649036 @default.
• W4385442606 cites W3186929771 @default.
• W4385442606 cites W3187888768 @default.
• W4385442606 cites W3195795879 @default.
• W4385442606 cites W3196401142 @default.
• W4385442606 cites W3196457189 @default.
• W4385442606 cites W4200184261 @default.
• W4385442606 cites W4210538176 @default.
• W4385442606 cites W4224246878 @default.
• W4385442606 cites W4225523429 @default.
• W4385442606 cites W4300960264 @default.
• W4385442606 cites W4307515194 @default.
• W4385442606 cites W4312113956 @default.
• W4385442606 cites W4317493097 @default.
• W4385442606 cites W4317863100 @default.
• W4385442606 cites W4321080528 @default.
• W4385442606 cites W4353016841 @default.
• W4385442606 doi "https://doi.org/10.1021/jacs.3c05023" @default.
• W4385442606 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37526259" @default.
• W4385442606 hasPublicationYear "2023" @default.
• W4385442606 type Work @default.
• W4385442606 citedByCount "0" @default.
• W4385442606 crossrefType "journal-article" @default.
• W4385442606 hasAuthorship W4385442606A5012950953 @default.
• W4385442606 hasAuthorship W4385442606A5014586466 @default.
• W4385442606 hasAuthorship W4385442606A5032221523 @default.
• W4385442606 hasAuthorship W4385442606A5064527448 @default.
• W4385442606 hasConcept C121332964 @default.
• W4385442606 hasConcept C127413603 @default.
• W4385442606 hasConcept C130349721 @default.
• W4385442606 hasConcept C147789679 @default.
• W4385442606 hasConcept C150394285 @default.
• W4385442606 hasConcept C17525397 @default.
• W4385442606 hasConcept C178790620 @default.
• W4385442606 hasConcept C179104552 @default.
• W4385442606 hasConcept C179366358 @default.
• W4385442606 hasConcept C185592680 @default.
• W4385442606 hasConcept C207740977 @default.
• W4385442606 hasConcept C2777379063 @default.
• W4385442606 hasConcept C32236832 @default.
• W4385442606 hasConcept C52859227 @default.
• W4385442606 hasConcept C544153396 @default.
• W4385442606 hasConcept C62520636 @default.
• W4385442606 hasConcept C68801617 @default.
• W4385442606 hasConcept C78519656 @default.
• W4385442606 hasConceptScore W4385442606C121332964 @default.
• W4385442606 hasConceptScore W4385442606C127413603 @default.
• W4385442606 hasConceptScore W4385442606C130349721 @default.
• W4385442606 hasConceptScore W4385442606C147789679 @default.
• W4385442606 hasConceptScore W4385442606C150394285 @default.
• W4385442606 hasConceptScore W4385442606C17525397 @default.
• W4385442606 hasConceptScore W4385442606C178790620 @default.
• W4385442606 hasConceptScore W4385442606C179104552 @default.
• W4385442606 hasConceptScore W4385442606C179366358 @default.
• W4385442606 hasConceptScore W4385442606C185592680 @default.
• W4385442606 hasConceptScore W4385442606C207740977 @default.
• W4385442606 hasConceptScore W4385442606C2777379063 @default.
• W4385442606 hasConceptScore W4385442606C32236832 @default.
• W4385442606 hasConceptScore W4385442606C52859227 @default.
• W4385442606 hasConceptScore W4385442606C544153396 @default.
• W4385442606 hasConceptScore W4385442606C62520636 @default.
• W4385442606 hasConceptScore W4385442606C68801617 @default.
• W4385442606 hasConceptScore W4385442606C78519656 @default.
• W4385442606 hasFunder F4320321001 @default.
• W4385442606 hasFunder F4320330241 @default.

• next