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• W4385442746 abstract "Manufacturing electrochemiluminescence (ECL) electrodes to detect analytes with high performance in the aqueous phase for water-insoluble metal complexes is a great challenge. Here, a directional self-assembling avenue for in situ fabricating iridium(III)-polyimine complex-encapsulated metal–organic framework (MOF) two-dimensional electrode Hf-MOF/Ir2PD/APS/ITO is developed. The electrode displayed bright red ECL emission with high stability in the aqueous phase and specific adsorption toward ssDNA against dsDNA and mNs. That is to say, a “high-performance and multifunctional ECL electrode” is presented and explored for sensitive detection of acetamiprid (Ace) with a limit of detection of 0.0025 nM, where Ace-aptamer recognition-switched Exonuclease III-mediated digestion to make large numbers of Fc-labeled ssDNA transform into Fc-mNs. Furthermore, the proposed method was triumphantly employed to monitor the change in the residual concentration of Ace in pakchoi. This work breaks through the bottleneck of metal complex-based ECL emission in organic solvents and provides a novel strategy to develop high-performance ECL sensors." @default.
• W4385442746 created "2023-08-02" @default.
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• W4385442746 date "2023-08-01" @default.
• W4385442746 modified "2023-10-11" @default.
• W4385442746 title "Directionally In Situ Self-Assembled Iridium(III)-Polyimine Complex-Encapsulated Metal–Organic Framework Two-Dimensional Nanosheet Electrode To Boost Electrochemiluminescence Sensing" @default.
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• W4385442746 doi "https://doi.org/10.1021/acs.analchem.3c01882" @default.
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