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• W4385582945 endingPage "124734" @default.
• W4385582945 startingPage "124734" @default.
• W4385582945 abstract "The stability of catalytic membrane reactors (CMRs) is crucial for the practical applications in chemical reaction processes. However, currently reported CMRs with perovskite-based oxygen permeable membranes usually show poor stability owing to the over-reduction of Co and Fe ions in perovskite lattice under harsh reducing gas atmospheres and the interaction between membrane and catalyst. Here we developed an oxygen permeable membrane Ce0.9Gd0.1O2-δ-SrCe0.5Fe0.5O3-δ (CGO-SCF) with Ce0.9Gd0.1O2-δ (CGO) protective layer to construct a catalytic membrane reactor packed with Ni/Al2O3 catalyst for partial oxidation of methane. The CGO dense protective layer can effectively avoid the over-reduction of Fe ions in perovskite under harsh reducing gas atmospheres and the interaction between perovskite and Ni/Al2O3. Benefiting from high stability and mixed ionic-electronic conductivity of CGO in a low oxygen partial pressure environment, the developed membrane reactor with a dense CGO thin film was successfully operated with a stable CH4 conversion of 87% and a H2/CO ratio of 2 over 200 h in harsh operating conditions. This strategy proposed here provides insights into the design of highly stable catalytic membrane reactor in harsh conditions." @default.
• W4385582945 created "2023-08-05" @default.
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• W4385582945 date "2023-11-01" @default.
• W4385582945 modified "2023-10-12" @default.
• W4385582945 title "Stable oxygen permeable membrane with Ce0.9Gd0.1O2-δ protective layer for syngas production" @default.
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• W4385582945 doi "https://doi.org/10.1016/j.seppur.2023.124734" @default.
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