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- W4385616968 abstract "Anion exchange membrane (AEM) water electrolysis is a promising technology for hydrogen production from renewable energy sources. However, the bottle-neck of its development is the poor comprehensive performance of AEM, especially the stability at high concentrated alkaline condition and temperature. Herein, we propose a new cationic group N-methylquinuclidinium with enhanced alkaline stability and hereby a full-carbon chain poly(aryl quinuclidinium) AEM was prepared. Compared with reported AEMs, it shows ultra-high comprehensive alkaline stability (no chemical decomposition, no decay of conductivity) in 10 M NaOH aqueous solution at 80°C for more than 1800 h, excellent dimensional stability (swelling ratio: < 10% in pure water, < 2% in 10 M NaOH) in OH- form at 80°C, high OH- conductivity (∼139.1 mS/cm at 80°C) and high mechanical properties (tensile strength: 41.5 MPa, elongation at break: 50%). The water electrolyser using our AEM exhibits a high current density (1.94 A/cm2 at 2.0 V) when assembled with nickel-alloy foam electrodes, and high durability when assembled with nickel foam electrodes. This article is protected by copyright. All rights reserved." @default.
- W4385616968 created "2023-08-07" @default.
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- W4385616968 date "2023-08-07" @default.
- W4385616968 modified "2023-10-16" @default.
- W4385616968 title "N‐Methylquinuclidinium Based Anion Exchange Membrane with Ultra‐High Alkaline Stability" @default.
- W4385616968 doi "https://doi.org/10.1002/adma.202306675" @default.
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- W4385616968 hasPublicationYear "2023" @default.
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