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- W4385657427 abstract "Aqueous zinc-ion batteries have been considered a potential substitute for lithium-ion batteries, due to its various advantages of abundant raw materials, high specific capacity and eco-friendliness. Among various anode materials, Zn metal is a promising anode of aqueous zinc-ion batteries owing to its high volumetric capacity, low cost and low redox potential. However, zinc metal anode suffers from serious problems of unrestricted dendritic growth and hydrogen production with electrolyte, resulting in capacity loss, decreased cycling performance, or even internal short circuit and battery failure. Herein, we modified zinc foil surface with CeO2-doped Polyethylene Oxide (PEO) thin film, which could effectively isolate aqueous electrolyte and zinc metal anode electrodes, and inhibit dendritic growth. In addition, theoretical calculations showed that after CeO2 doping, the band gap of the modified was reduced, which promoted the transport of Zn2+ and improved the diffusion coefficient of zinc ions. With the above synergistic effect of engineered PEO, the Zn‖Zn symmetrical cells delivered a stable cycle of 2690 h at a current of 1 mA cm−2. Moreover, this study provides technical support for the further large-scale use of aqueous zinc-ion batteries." @default.
- W4385657427 created "2023-08-09" @default.
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- W4385657427 date "2023-12-01" @default.
- W4385657427 modified "2023-10-16" @default.
- W4385657427 title "Achieving dendrite-free and long cyclic stability of zinc anode via CeO2 doped PEO interface modification" @default.
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- W4385657427 doi "https://doi.org/10.1016/j.fuel.2023.129417" @default.
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