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- W4385703100 abstract "Fabricating stable MOF membranes with high permeance for H2 separation and purification faces significant challenges primarily due to the heterogeneous nucleation of MOF on substrate. Herein, we propose a simple but effective homoelemental strategy by choosing the Zn-based ZIF-8 and Zn foam substrate. Without any chemical or physical modification, a serials of highly stable and compact ZIF-8 membranes are assembled on the Zn foam which exhibit high H2 permeance both for H2/CH4 and H2/CO2 separation. Especially, the 1-Zn-Foam/ZIF-8-24 membrane displays the high H2 permeance close to 104 GPU, surpassing most MOF membranes for H2/CH4 and H2/CO2 separation. Further, the excellent stability displays steady H2 permeance and selectivity, even after 96-hour testing, high temperature of 100 oC, or high pressure. This is the first exploration by adopting Zn foam as a substrate for gas separation, not only demonstrating the Zn foam is an ideal carrier for assembling the Zn-based MOF membranes, but also implying the potential of the homoelemental strategy in fabricating other MOF membranes." @default.
- W4385703100 created "2023-08-10" @default.
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- W4385703100 date "2023-11-01" @default.
- W4385703100 modified "2023-10-12" @default.
- W4385703100 title "Homoelemental effect boosted stable ZIF-8 membrane with super high H2 permeance" @default.
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- W4385703100 doi "https://doi.org/10.1016/j.seppur.2023.124751" @default.
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