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- W4385703329 abstract "The selective functionalization of unreactive C–H bonds over reactive polar functionalities paves the way for the efficient synthesis of complex molecular frameworks. Here, we report a consecutive C–H alkylation and Wittig-type reaction of phosphorus ylides, enabling the conversion of inert C–H and C=P bonds into C–C and C=C bonds, respectively. Under blue-light irradiation and with the aid of an appropriate photoredox catalyst, a mixture encompassing phosphorus ylides, electron-rich olefins, and unsaturated carbonyl compounds adeptly undergoes a previously elusive three-component cycloaddition. This transformation allows for the rapid construction of the synthetically versatile functionalized six-membered carbocycles from readily available substrates." @default.
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- W4385703329 date "2023-08-09" @default.
- W4385703329 modified "2023-09-26" @default.
- W4385703329 title "Catalytic Formal Carbyne Transformation of Phosphorus Ylides" @default.
- W4385703329 doi "https://doi.org/10.26434/chemrxiv-2023-mx0vg" @default.
- W4385703329 hasPublicationYear "2023" @default.
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