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• W4385715960 abstract "Exploration of new functional materials with enhanced performance from known ones is always an attractive strategy. A new infrared (IR) nonlinear-optical (NLO) mixed chalcogenide Ag2In2SiS3.06Se2.94 (1), was obtained through partial congener substitution originated from Ag2In2SiS6 (0). 1 crystallizes in the monoclinic space group Cc, and its three-dimensional (3D) polyanionic network is composed of {[In4Si2Se5(S/Se)11]12–}∞ helical chains sharing S/Se(5) corner atoms with cavities embedded with counterion Ag+ ions. It exhibits a much enhanced NLO response compared to that of 0, reaching 1.1 × AgGaS2. Further theoretical analysis results indicate that the large NLO response can be attributed to the synergistic effect of AgQ4 and InQ4 tetrahedral functional motifs. This work not only reports a new high-performance IR NLO material but also enriches the partial ion substitution strategy to obtain new functional materials." @default.
• W4385715960 created "2023-08-11" @default.
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• W4385715960 date "2023-08-10" @default.
• W4385715960 modified "2023-09-26" @default.
• W4385715960 title "Three-in-One Tetrahedral Functional Units Constructing Diamondlike Ag₂In₂SiS_3.06Se_2.94 with High-Performance Nonlinear-Optical Activity" @default.
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• W4385715960 doi "https://doi.org/10.1021/acs.inorgchem.3c02369" @default.
• W4385715960 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37560964" @default.
• W4385715960 hasPublicationYear "2023" @default.
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