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- W4385721167 abstract "Three-dimentional (3D) transition metal selenides with sufficient channels could produce significant superiority on enhancing reaction kinetics for sodium-ion batteries. However, the thorough exploration of 3D architecture with a facile strategy is still challenging. Here we report that a polycrystalline Cu2-xSe film was epitaxial grown on (220) facets-exposed Cu by direct selenization of a nanoporous Cu skeleton, which is obtained by dealloying rolled CuMn@Cu alloy foil. Density Functional Theory calculation result shows strong adsorption energy for Se atoms on Cu (220) planes during selenization reaction, rendering a low energy consumption. By virtue of this core-shell 3D nanoporous architecture to offer abundant active sites and endow fast electron/ion transportation, the nanoporous Cu2-x[email protected] composite electrode exhibits remarkable sodium-ion storage properties with high reversible capacity of 950.6 μAh/cm2 at 50 μA/cm2, suprior rate capability of 457.6 μAh/cm2 at 500 μA/cm2, as well as an ultra-long stability at a high current density. Mechanism investigation reveals that the electrochemical reaction is a typical conversion-type reaction with different intermediates. This novel electrode synthetic strategy provides useful instructions to design the high-performance anode material for sodium-ion batteries." @default.
- W4385721167 created "2023-08-11" @default.
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- W4385721167 date "2023-08-01" @default.
- W4385721167 modified "2023-10-15" @default.
- W4385721167 title "Epitaxial growth of Cu2-xSe on Cu (220) crystal plane as high property anode for sodium storage" @default.
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- W4385721167 doi "https://doi.org/10.1016/j.cclet.2023.108922" @default.
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