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• W4385755648 abstract "Frame/skeleton-like nanostructures are of great value in plasmonic catalysis as a result of the synergetic structural advantages arising from both maximized surface atomic exposure and efficient incident light absorptions. Herein, we report the size-tunable fabrication of yolk-shell AuAg nanoparticles containing a spherical core and cuboctahedral skeletons (AuAg YSCNSs), together with the exploration of their applications for assisting the reduction of 4-nitrophenol (4-NP) under ultraviolet-visible (UV-vis) light irradiation. The use of glutathione (GSH) at an appropriate amount to mediate the galvanic replacement reaction between Au@Ag core-shell nanocubes and HAuCl4 is found to be crucial in regulating the shape evolution. Their sizes could be readily tuned by altering the edge lengths of Au@Ag core-shell nanocubes. When working as the photocatalyst assisting the reduction of 4-NP, the AuAg YSCNSs exhibit a higher apparent rate constant under UV-vis light irradiation. The current work demonstrates the feasibility to create skeleton-like noble metal nanocrystals with the shape largely deviated from that of the original template via the top-down carving strategy by introducing non-metallic surface doping, which could be potentially extended to other noble metals or alloys." @default.
• W4385755648 created "2023-08-12" @default.
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• W4385755648 date "2023-08-11" @default.
• W4385755648 modified "2023-10-16" @default.
• W4385755648 title "Glutathione-Mediated Synthesis of Yolk–Shell AuAg Nanostructures Containing a Spherical Core and Cuboctahedral Skeletons and Their Applications in Plasmonic Catalysis" @default.
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• W4385755648 doi "https://doi.org/10.1021/acs.langmuir.3c01506" @default.
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