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• W4385767016 abstract "Abstract Diffusion is a fundamental irreversible process intervening in the evolution of many out-of-equilibrium systems and is successfully described by Fick’s law obtained from non-equilibrium thermodynamics. Despite this, numerical simulations of solid state electro-deoxidation in the diffusion-controlled regime in molten salt remain elusive. Here, a new model for diffusion controlled three-phase interline (3PI) penetration in a porous cathode during electro-deoxidation is validated against experimental observation. This penetrating 3PI model is applied at high overpotential and benchmarked using the oxygen ionisation TiO 2 (s) + 4e − → Ti(s) + 2O 2− at the 3PI. The model couples slow diffusive transport and fast oxygen ionisation while assuming a negligible ohmic potential drop in bulk molten CaCl 2 electrolyte. The 14 nm s −1 penetration rate of the 3PI and the order of magnitude of 3PI currents (derived from an exchange current density and cathodic transfer coefficient of 0.32 A cm −2 and 0.01, respectively) in the chronoamperometric data for porous cathodes are in good agreement with experimental observation." @default.
• W4385767016 created "2023-08-12" @default.
• W4385767016 creator A5015035636 @default.
• W4385767016 creator A5050782013 @default.
• W4385767016 date "2023-08-11" @default.
• W4385767016 modified "2023-10-18" @default.
• W4385767016 title "Modelling diffusion controlled electro-deoxidation of metal oxide to metal in molten salt" @default.
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• W4385767016 doi "https://doi.org/10.1007/s10008-023-05624-5" @default.
• W4385767016 hasPublicationYear "2023" @default.
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