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- W4385808230 abstract "Abstract Despite the potentially higher energy density and improved safety of solid-state batteries (SSBs) relative to Li-ion batteries, failure due to Li-filament penetration of the solid electrolyte and subsequent short circuit remains a critical issue. Herein, we show that Li-filament growth is suppressed in solid-electrolyte pellets with a relative density beyond ~ 95%. Below this threshold value, however, the battery shorts more easily as the density increases due to faster Li-filament growth within the percolating pores in the pellet. The microstructural properties (e.g., pore size, connectivity, porosity, and tortuosity) of 75% Li 2 S - 25 P 2 S 5 with various relative densities are quantified using focused ion beam–scanning electron microscopy tomography and permeability tests. Furthermore, modeling results provide details on the Li-filament growth inside pores ranging from 0.2 to 2 µm in size. Our findings improve the understanding of the failure modes of SSBs and provide guidelines for the design of dendrite-free SSBs." @default.
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- W4385808230 date "2023-08-14" @default.
- W4385808230 modified "2023-10-16" @default.
- W4385808230 title "Effect of Solid-Electrolyte Pellet Density on Failure of Solid-State Batteries" @default.
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- W4385808230 doi "https://doi.org/10.21203/rs.3.rs-3246916/v1" @default.
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